6–8 Jun 2011
Columbia University
US/Eastern timezone
AICI (June 6-7, 2011) and Snow Chemistry Modeling (June 8, 2011) workshops

Model simulations of polar boundary layer ozone depletion events in spring

6 Jun 2011, 12:05
1h 10m
Columbia University

Columbia University

New York, NY, USA

Speaker

Dr Xin Yang (University of Cambridge)

Description

In the last several decades, significant depletion of boundary layer ozone (ODEs) has been observed in both Antarctic and Arctic, especially over sea ice zones. ODEs are attributed to catalytic destruction by bromine radicals (Br and BrO), especially during bromine explosion events (BEs), when high concentrations of BrO periodically occur. However, neither the exact source of the bromine nor the mechanism of the formation of ODEs is completely understood. Here, by considering an additional bromine source from sea ice (through blowing snow events), we can successfully reproduce some of observed BEs in a 3D global transport model, pTOMCAT. Modelled tropospheric BrO compares well, in general, with the tropospheric BrO column retrieved from the GOME satellite instrument. Observed surface ozone data , e.g. at Halley, are also compared with the simulations to further validate the mechanism of bromine release and investigate the condition for surface ODEs. Cases with large BEs over Weddell Sea are chosen for specific comparison.

Please list some keywords

Model ozone depletion bromine explosion blowing-snow

Primary author

Dr Xin Yang (University of Cambridge)

Co-authors

Dr Anna Jones (British Antarctic Survey) Prof. John Pyle (University of Cambridge)

Presentation materials

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