4–6 Apr 2011
ETH Zurich, Campus Science City, HIT Building
Europe/Zurich timezone

Novel Quadratic X-Ray Magneto-Optical Effect for Time-resolved Experiments at the M Edges of the 3d Transition Metals

4 Apr 2011, 16:30
2h 30m
ETH Zurich, Campus Science City, HIT Building

ETH Zurich, Campus Science City, HIT Building

Speaker

Armin Kleibert (Swiss Light Source, Paul Scherrer Institut, CH-5232 Villigen, Switzerland)

Description

We have observed a quadratic x-ray magneto-optical effect in near-normal-incidence reflection at the M edges of iron [1]. The effect appears as the magnetically induced rotation of ~0.1° of the polarization plane of linearly polarized x-ray radiation upon reflection. A comparison of the measured rotation spectrum with results from x-ray magnetic linear dichroism data demonstrates that this is the first observation of the Schaefer-Hubert effect in the x-ray regime. Ab initio density-functional theory calculations reveal that hybridization effects of the 3p core states necessarily need to be considered when interpreting experimental data. The discovered magneto-x-ray effect holds promise for future ultrafast and element-selective studies of ferromagnetic as well as antiferromagnetic materials. [1] S. Valencia, A. Kleibert, A. Gaupp, J. Rusz, D. Legut, J. Bansmann, W. Gudat, and P. M. Oppeneer, Phys. Rev. Lett. 104, 187401 (2010)

Author

Armin Kleibert (Swiss Light Source, Paul Scherrer Institut, CH-5232 Villigen, Switzerland)

Co-authors

Andreas Gaupp (Helmholtz-Zentrum-Berlin, BESSY, Albert-Einstein-Straße 15, D-12489 Berlin, Germany) Dominik Legut (Department of Physics and Materials Science, Uppsala University, Box 530, S-751 21 Uppsala, Sweden) Jan Rusz (Department of Physics and Materials Science, Uppsala University, Box 530, S-751 21 Uppsala, Sweden) Joachim Bansmann (Institute of Surface Chemistry and Catalysis, Universitaet Ulm, D-89069 Ulm, Germany) Peter Oppeneer (Department of Physics and Materials Science, Uppsala University, Box 530, S-751 21 Uppsala, Sweden) Sergio Valencia (Helmholtz-Zentrum-Berlin, BESSY, Albert-Einstein-Straße 15, D-12489 Berlin, Germany) Wolfgang Gudat (Helmholtz-Zentrum-Berlin, BESSY, Albert-Einstein-Straße 15, D-12489 Berlin, Germany)

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