18–20 Sept 2013
Paul Scherrer Institut, Villigen, Switzerland
Europe/Zurich timezone

Magnetic excitations in the Ising-chain material RbCoCl3

19 Sept 2013, 12:30
2h
WSLA - Foyer (Paul Scherrer Institut, Villigen, Switzerland)

WSLA - Foyer

Paul Scherrer Institut, Villigen, Switzerland

Board: 81

Speaker

Ms Eva Hirtenlechner (Institut Laue Langevin, BP 156, 38042 Grenoble Cedex 9, France, Laboratory for Neutron Scattering, Paul Scherrer Institute, CH-5232 Villigen PSI, Switzerland)

Description

One of the simplest realizations of a quantum phase transition is the Ising model in a transverse magnetic field. The Co2+ ion is a good resource for anisotropic spins with Ising or XY interactions. Several families of cobalt halides and oxides have been classified as approximate realizations of the Ising chain model. The hexagonal perovskite family ACoX3 with A = Rb, Cs, Tl and X = Br, Cl is one class of potential Ising materials [1, 2, 3]. The material RbCoCl3 has been studied to a lesser extent. In RbCoCl3 the Co2+ ions have effective spin-½. Neutron powder diffraction data show that the ordered magnetic moments are aligned antiferromagnetically up-down the crystallographic c-axis with an amplitude modulation in the ab-plane. Two antiferromagnetic phase transitions at TN1 = 28 K and TN2 = 13 K were observed [4]. On the new thermal TAS EIGER at SINQ, the spectrometer IN22 at ILL and the LET ToFspectrometer at ISIS Ising-domain wall excitations were measured. These excitations show a cosinusoidal dispersion and sharpening and splitting at the successive magnetic transitions at TN1 and TN2. In the experiment on we observed how the excitations change with temperature. We were also able to observe the splitting of the modes in a very successful commissioning experiment on EIGER at PSI. We will present results and preliminary analysis of the LET, IN22 and EIGER data. References [1] S. Nagler et al., Phys. Rev. Lett. 49, 590 (1982). [2] J. Goff et al., Phys. Rev. B 52, 15992 (1995). [3] A. Oosawa et al., J. Phys. Soc. Jpn. 75, 015002 (2006). [4] N. Hänni et al., in preparation.

Primary author

Ms Eva Hirtenlechner (Institut Laue Langevin, BP 156, 38042 Grenoble Cedex 9, France, Laboratory for Neutron Scattering, Paul Scherrer Institute, CH-5232 Villigen PSI, Switzerland)

Co-authors

Prof. Christian Rüegg (Laboratory for Neutron Scattering, Paul Scherrer Institute, CH-5232 Villigen PSI, Switzerland, DPMC-MaNEP, University of Geneva, CH-1211 Geneva, Switzerland) Prof. Des McMorrow (London Centre for Nanotechnology, University College London, LondonWC1E 6BT, UK) Dr Karl Krämer (Department of Chemistry and Biochemistry, University of Bern, CH-3012 Bern, Switzerland) Dr Louis-Pierre Regnault (CEA-Grenoble, DRFMC-SPSMS-MDN, Grenoble Cedex 9, France) Mr Mattia Mena (London Centre for Nanotechnology, University College London, LondonWC1E 6BT, UK, Laboratory for Neutron Scattering, Paul Scherrer Institute, CH-5232 Villigen PSI, Switzerland) Ms Nora Hänni (Universität Bern) Dr Robert Bewley (ISIS Facility, Rutherford Appleton Laboratory, Chilton, Didcot OX11 0QX, UK) Dr Uwe Stuhr (Laboratory for Neutron Scattering, Paul Scherrer Institute, CH-5232 Villigen PSI, Switzerland)

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